Izvestiya vuzov. Yadernaya Energetika

The peer-reviewed scientific and technology journal. ISSN: 0204-3327

Neutronic Foundations for Large-Scale Production of 238Pu for Independent Energy Sources

6/22/2023 2023 - #02 Physics in nuclear power engineering

Kulikov G.G. Shmelev A.N. Glebov V.B. Apse V.A. Kulikov E.G.

DOI: https://doi.org/10.26583/npe.2023.2.13

UDC: 621.039.8

The paper considers the neutronic foundations for large-scale production of 238Pu for independent energy sources. The 238Pu isotope is a unique source of long-term independent energy supply in various devices for remote areas on Earth and in space. At the same time, the capacity for its production currently available in Russia and worldwide is insufficient.

The paper considers the chains for producing the 238Pu isotope and defines the optimal spectrum and neutron flux for its production. A conclusion is made that the most attractive starting isotope is 237Np that can be extracted from irradiated nuclear fuel. The proposed method allows for large-scale production of plutonium, which is distinctive in high content of the 238Pu isotope and low content of the 236Pu isotope.

References

  1. US Department of Energy Start Up Plan for Plutonium 238 Production for Radioisotope Power Systems. Available at: https://www.energy.gov/sites/default/files/2015/09/f26/Final_Startup_Plan_for_Plutonium238.pdf (accessed Nov. 10, 2022).
  2. An Exploration of Mission Concepts that Could Utilize Small RPS. Available at: http://anstd.ans.org/NETS-2019-Papers/Track-2–Mission-Concepts-and-Logistics/abstract-31-0.pdf (accessed Nov. 10, 2022).
  3. INFCIRC/153. The Structure and Content of Agreements Between the Agency and States Required in Connection with the Treaty on the Non Proliferation of Nuclear Weapons. Available at: https://www.iaea.org/sites/default/files/publications/documents/infcircs/1972/infcirc153.pdf (accessed Nov. 10, 2022).
  4. Shmelev A.N., Geraskin N.I., Kulikov G.G., Kulikov E.G., Apse V.A., Glebov V.B. The Problem of Large Scale Production of Plutonium 238 for Autonomous Energy Sources. Journal of Physics: Conference Series. 2020, v. 1689, iss. 111, paper no. 012030; DOI: https://doi.org/10.1088/17426596/1689/1/012030 .
  5. Shibata K., Iwamoto O., Nakagawa T., Iwamoto N, Ichihara A., Kunieda S., Chiba S., Furutaka K, Otuka N., Ohsawa T., Murata T., Matsunobu H., Zukeran A., Kamada S. & Katakura J. JENDL 4.0: A New Library for Nuclear Science and Engineering. Journal of Nuclear Science and Technology. 2011, v. 48(1), pp. 1 30.
  6. Radioisotope Power Systems for Deep Space Exploration – Some Background. Available at: https://www.nationalacademies.org/event/03-05-2021/docs/-D7D82520CDCFA8423E16CD569643B93B8837DDEA9EDB (accessed Nov. 10, 2022).
  7. Daily C.R., McDuffee J.L. Design Studies for the Optimization of 238Pu Production in NpO2 Targets Irradiated at the High Flux Isotope Reactor. Nuclear Technology. 2020, v. 206. pp. 1182 1194; DOI: https://doi.org/10.1080/00295450.2019.1674594 .
  8. The Experience of Military Hydrographers of the Russian Federation can Speed up the Cleaning of the Northern Sea Route from RTGs – Expert. Available at: http://www.atominfo.ru/news9/i0545.htm (accessed Nov. 10, 2022) (in Russian).
  9. The Pentagon Ran out of Russian Plutonium. Available at: https://lenta.ru/articles/-2005/06/28/plutonium/ (accessed Nov. 10, 2022) (in Russian).
  10. The Mayak Plant Began Designing the Latest Research Reactor. Available at: https://tass.ru/ural-news/2304431 (accessed Nov. 10, 2022) (in Russian).
  11. Optimization of Plutonium 238 Production in the Advanced Test Reactor for Radioisotope Thermoelectric Generators in Deep Space Exploration Applications. Available at: https://www.researchgate.net/publication/332182780 (accessed Nov. 10, 2022).
  12. Betzler B.R., Chandler D., Evans T.M., Davidson G.G., Daily C.R., Wilson S.C., Mosher S.W. As Built Simulation of the High Flux Isotope Reactor. Journal of Nuclear Engineering. 2021. Vol. 2. PP. 28–34. DOI: https://doi.org/10.3390/jne2010003.
  13. Process Development for Plutonium 238 Production at Oak Ridge National Laboratory. Available at: http://anstd.ans.org/NETS-2019-Papers/Track-5–-Radioisotope-Power-Systems/abstract-80-0.pdf (accessed Nov. 10, 2022).

238Pu nuclide transformation chains 237Np

Link for citing the article: Kulikov G.G., Shmelev A.N., Glebov V.B., Apse V.A., Kulikov E.G. Neutronic Foundations for Large-Scale Production of 238Pu for Independent Energy Sources. Izvestiya vuzov. Yadernaya Energetika. 2023, no. 2, pp. 162-168; DOI: https://doi.org/10.26583/npe.2023.2.13 (in Russian).